Sure, “arbitrary” is a suitable term here too. A random process is just one way to generate an arbitrary function.
My use of “random” here was referring to the coin flipping process and was more for building intuition than precisely specifying all the other non-expressible functions. I was trying to allude to the fact that these other type of functions don’t have any easily expressible process behind them. When I’ve taught this stuff in the past I’ve found that people latch onto coin flipping more easily that imagining some arbitrary assignment of values.
For what it’s worth, I used to be a researcher in probability and information theory and have published papers on those topics so I am aware of the various technical definitions of randomness (Kolmogorov axioms, algorithmic probability theory, etc.)
I think you’re right about my comment being a little too lengthy for most people to find useful. I started explaining this stuff and got carried away.